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Magnetic Field-Enhanced Graphene Superconductivity with Record Pauli-Limit Violation

Authors

  • Jixiang Yang
  • Omid Sharifi Sedeh
  • Chiho Yoon
  • Shenyong Ye
  • Henok Weldeyesus
  • Armel Cotten
  • Tonghang Han
  • Zhengguang Lu
  • Zach Hadjri
  • Junseok Seo
  • Lihan Shi
  • Emily Aitken
  • Prayoga P Liong
  • Zhenghan Wu
  • Mingchi Xu
  • Christian Scheller
  • Mingyang Zheng
  • Rasul Gazizulin
  • Kenji Watanabe
  • Takashi Taniguchi
  • Dominique Laroche
  • Mingda Li
  • Fan Zhang
  • Dominik M. Zumbühl
  • Long Ju

Abstract

Spin-polarized superconductors offer a rare platform for studying electronic correlations, but few candidate systems have been experimentally confirmed to date. Here, we report the observation of a spin-polarized superconducting state, denoted SC5, in WSe2-proximitized rhombohedral trilayer graphene. At in-plane magnetic field B|| = 0 T, SC5 has a critical temperature of 68 mK and an out-of-plane critical magnetic field of only 12 mT. Surprisingly, these values are significantly enhanced as B|| increases, and the superconductivity persists to B|| = 8.8 T. This value corresponds to a record-high Pauli-limit violation ratio of at least 80 among all superconductors, while the true critical field is beyond the limit of our instrument. We conclude that SC5 experiences a canting crossover from Ising-type to spin-polarized superconductor with increased B||.

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Posted

2025-11-22